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Highly selective, catalyst-free CO2 reduction in strong acid without alkali cations by a mechanical energy-induced triboelectric plasma-electrolytic system
DOI: 10.1039/D5GC00977D, CommunicationHui Hu, Nannan Liu, Qinglong Ru, Wei Jiang, Yongcui Yang, Kailan Ma, Lixiang Meng, Zuliang Du, Bao Zhang, Gang Cheng
A mechanical energy-driven hybrid triboelectric plasma-electrochemical system in strong acids was constructed to trigger CO2 reduction at room temperature and atmospheric pressure without catalysts or alkali cations.
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Building a multifunctional Cu2Se@biomass carbon composite interfacial layer on a zinc anode for stable aqueous zinc-ion batteries
DOI: 10.1039/D5GC01034A, PaperWenjing Zheng, Tieran Zhou, Hao Zhou, Jie Guan, Fei Wang, Lin Zhu, Zhongti Sun, Kan Zhang
Cu2Se@BC was constructed to improve the structural stability of Zn anodes. It can induce the preferential orientation of zinc ions on the Zn (002) crystal plane. The AZIBs assembled with the Cu2Se@BC–Zn anode showed good electrochemical performance.
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Gentle and rapid synthesis of imine-linked covalent organic frameworks in acetic acid-based deep eutectic solvents
DOI: 10.1039/D5GC01800E, PaperQuanyuan Qiu, Guanwei Li, Chenxi Shi, Yueren Zeng, Kunchi Xie, Ke Wang, Zhen Song, Zhenjie Zhang, Xiaoqing Lin
Using natural green menthol/AA DES as both solvent and catalyst for the rapid synthesis of more than 20 highly crystalline imine-linked COFs with varying structures under mild conditions.
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Water-assisted diboron activation: efficient synthesis of alkyl 1,2-bis(boronates) and 1,1,2-tris(boronates)
DOI: 10.1039/D5GC00743G, PaperKiran S. Patil, Shivakumar Reddappa, Maruti Suryavansi, Srinivasa Budagumpi, D. H. Nagaraju, Manoj V. Mane, Shubhankar Kumar Bose
A simple, efficient, and environmentally benign method for the synthesis of alkyl 1,2-bis(boronates) and 1,1,2-tris(boronates) from diboration and triboration of alkenes and alkynes has been developed via water-assisted diboron activation.
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Bio-waste derived Ni single-atom catalysts with Ni-pyridine-N4 active sites for efficient N-alkylation of alcohols and amines
DOI: 10.1039/D5GC00434A, PaperYuxin Zhu, Qiudi Zhu, Youjuan Tan, Hongqin Wang, Xuefei Liu, Wei Gong, Dongdong Ye, Xianglin Pei
Chitin derived from seafood waste is used as raw materials to fabricate Ni SACs. The synthetic catalyst exhibits excellent catalytic performance in N-alkylation of alcohols with amines, as well as good stability and broad substrate compatibility.
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Oxidized thiourea derivatives: uncovering new frontiers with resonant acoustic mixing (RAM)
DOI: 10.1039/D4GC06064D, PaperPietro Caboni, Francesco Basoccu, Shyamal Kanti Bera, Andrea Porcheddu
Nitrogen-containing compounds are essential for producing active pharmaceutical ingredients.
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Novel arylindane diols as sustainable primary antioxidants from lignin
DOI: 10.1039/D4GC05190D, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Tessy Hendrickx, Laura Trullemans, Alexander J. Heyer, Imke Boonen, Marko Turkalj, Fatima Rammal, Yiqi Su, Besarta Matranxhi, Durgasruthi Pully, Bart Van Meerbeek, Peter Van Puyvelde, Marc Elskens, Kirsten L. Van Landuyt, Bert F. SelsA zeolite-catalyzed green synthesis of diisoeugenol. Together with diisoallylsyringol, these novel arylindane diols are safe and sustainable primary antioxidants.
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Electron-deficient Mo sites enhance electrochemical nitrate reduction to ammonia by promoting water dissociation
DOI: 10.1039/D5GC01249J, PaperXue Zhou, Wence Xu, Yunduo Huang, Zhonghui Gao, Yanqin Liang, Hui Jiang, Zhaoyang Li, Fang Wang, Shengli Zhu, Zhenduo Cui
Nanoporous Mo-doped Co2P exhibits outstanding NITRR performance, as the introduction of electron-deficient Mo promotes H2O dissociation to *H, enabling efficient NO hydrogenation with nearly 100% NH3 FE and 40.6% EE at −0.1 V vs. RHE.
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Synergism of tiny Ni clusters and Pt nanoparticles promoting efficient and stable electrocatalytic methanol oxidation and hydrogen evolution by water electrolysis
DOI: 10.1039/D5GC00992H, PaperJie Huang, Min Tian, Liang Tong, Lihua Zhu, Lingling Li, Xianping Liao, Qingsheng Gao, Weizhen Wang, Zhiqing Yang, Tongxiang Liang, Hengqiang Ye
This work illustrates that the synergistic effect of tiny Nics and PtNPs provides a novel strategy for designing highly active and durable electrocatalysts (Pt10/Ni-ZrO2-NC) for the MOR, HER and the coupling reaction of MOR∥HER.
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Engineered enzymatic cascade converts diols to amino alcohols
DOI: 10.1039/D4GC02141J, Paper
Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Hannah R. Valentino, Liangyu Qian, Jerry M. Parks, Erin E. Drufva, Ada Sedova, Pankti S. Mehta, Mary P. Watson, Richard J. Giannone, Stephanie S. Galanie, Joshua K. MichenerAliphatic amino alcohols such as 6-amino-1-hexanol are potential platform chemicals for a variety of advanced materials. Selective enzymatic synthesis from biomass-derived diols could simplify production while minimizing hazards.
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Metal-free carboxamidation of P(O)H compounds with in situ formed isocyanates from dioxazolones: a convenient access to carbamoylphosphine oxides
DOI: 10.1039/D5GC00470E, PaperYong Zhao, Longyang Chen, Guohao Xu, Shanshan Meng, Chuan Fu, Pengxiang Xu, Yuxing Gao, Yufen Zhao
A facile and metal-free method for synthesizing structurally diverse carbamoylphosphine oxides from dioxazolones and P(O)H compounds was developed.
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Radical click reaction for C–S bond construction via reductive coupling of phthalimide derivatives
DOI: 10.1039/D5GC01731A, PaperJia-Fan Qiao, Tian-Zhang Wang, Peng-Hui Shen, Yu-Qiu Guan, Ya-Xin Yu, Yu-Feng Liang
An efficient radical click reductive cross coupling with phthalimide derivatives has been established, which is characterized by simple conditions, good functional group compatibility without catalyst or ligands to construct C–S bond in two minutes.
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Green chemistry perspectives on click chemistry approaches for cellulose functionalization: a critical review
DOI: 10.1039/D5GC01227A, Critical ReviewBowen Li, Chaoqun Xu, Xinyi Zhu, Juan Yu, Xiaofang Zhang, Yimin Fan
Exploring green chemistry perspectives on click chemistry approaches for cellulose functionalization.
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Green innovations in C–H bond functionalisation: exploring homogeneous recyclable catalytic systems
DOI: 10.1039/D5GC00278H, Tutorial ReviewDewal S. Deshmukh, Sanjay Singh, Kirtikumar C. Badgujar, Vivek T. Humne, Gajanan V. Korpe, Bhalchandra M. Bhanage
This review focuses on homogeneous recyclable catalytic systems for direct C–H bond functionalization in organic synthesis, eliminating pre-functionalization. It explores recyclable catalysts with various metals and metal-free approaches.
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Metabolic channelling in Rhodopseudomonas palustris for diversification and sustainability assessment of polyhydroxyalkanoates
DOI: 10.1039/D4GC05663A, PaperPoonam Kumari, S. Venkata Mohan
Green metabolic channelling in Rhodopseudomonas palustris enables diverse PHA production from renewable substrates. Polymer profiling and sustainability assessment validate its biorefinery potential for eco-friendly plastic alternatives.
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Green reactions by metallosilicate catalysts
DOI: 10.1039/D5GC00086F, Tutorial ReviewHao Xu, Jie Tuo, Longkang Zhang, Yue Ma, Yejun Guan, Peng Wu
Metallosilicates feature framework-incorporated metal sites, serve as efficient catalysts for green selective oxidation reactions, and act as effective supports for confining precious metals in the conversion of low-carbon resources.
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Rational design of an efficient Pt3Cu/TiO2 icosahedral catalyst for bio-aviation fuel production under mild conditions
DOI: 10.1039/D5GC01235J, PaperYichen Nie, Xingyong Li, Misbah Uddin, Na Liu, Senshen Yu, Phidsavard Keomeesay, Olajide-rasheed Olalekan, Shuaizhe Li, Yubao Chen, Xuebing Zhao, Longlong Ma, Zhifeng Zheng, Shijie Liu
Icosahedral and octahedral structures can be obtained using hydrothermal preparation with only a change in the precursor. Pt3Cu/TiO2 icosahedra can be used to prepare bio-aviation fuel under mild conditions with 91.8% selectivity for target alkanes.
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Tandem electrocatalytic benzylic alcohol oxidation and aldol condensation for efficient valuable α,β-unsaturated ketone production
DOI: 10.1039/D5GC01155H, PaperYifan Yan, Xi Cai, Jiangrong Yang, Yu Fu, Qiwei Shi, Pengjie Hao, Hua Zhou, Zhenhua Li, Mingfei Shao, Haohong Duan
This study presents a one-step electrosynthesis method for α,β-unsaturated ketones using an Au/CuO cooperative catalyst for selective oxidation of aromatic alcohols followed by aldol condensation, achieving green and efficient production.
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Carbonized polymer dots as electrolyte additives for suppressing Zn dendrite growth, corrosion, and the HER in Zn-ion batteries
DOI: 10.1039/D5GC00702J, PaperXiao-Yan Shen, Guo-Duo Yang, Xin-Yao Huang, Yan-Fei Li, Zhuo Wang, Tong Wang, Ru-Yi Liu, Yi-Han Song, Ming-Xiao Deng, Hai-Zhu Sun
Low-cost, eco-friendly CPDs are designed and synthesized as electrolyte additives to effectively enhance the stability of aqueous ZIBs. This work offers significant advancement in the development of green and clean energy storage devices.
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Boosting NH3-SCR of NOx performance through sustainable and economical synthesis of Cu-SAPO-34 zeolites from attapulgite
DOI: 10.1039/D5GC01362C, PaperYao Wang, Zhangpei Liu, Yongjun Feng, Christopher Hardacre, Sarayute Chansai, Zhiming Liu
Cu-SAPO-34 has been synthesized using attapulgite, which not only demonstrates promising application potential but also introduces an innovative approach for designing cost-effective and active SCR catalysts using low-cost and abundant raw materials.
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