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Cesium chemistry enables microporous carbon nanofibers with biomimetic ion transport channels for zinc-ion capacitors
DOI: 10.1039/D5GC02376A, PaperZhenye Yin, Xuan Luo, Qian Zhang, Guangjie Yang, Chunmei Zhang, Zhenlu Liu, Xue Li, Jian Song, Haoqi Yang, Shuijian He
This work presents a sustainable “cesium chemistry” strategy to directly convert cellulose acetate into microporous carbon nanofibers with biomimetic ion channels, enabling efficient Zn2+ storage and high-performance zinc-ion capacitors.
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Ecotoxicity of binary mixtures of cholinium-based ionic liquids and salts to microalgae
DOI: 10.1039/D5GC02838H, Paper
Open Access 
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Fátima Jesus, Joana L. Pereira, Sónia P. M. Ventura, João A. P. Coutinho, Fernando J. M. Gonçalves, Ana M. M. GonçalvesMixtures of cholinium-based ILs and salts may pose lower environmental hazards than anticipated from the toxicities of their individual components.
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Dynamic tailoring gradient porosity of biomass-derived porous carbons for highly effective CO2 capture
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC03217B, PaperBinbin Chang, Weiwei Shi, Yanzhen Guo, Qixin Lu, Haitao Li, Yachao Liang, Faxue Ma, Baocheng Yang
Carbon capture has emerged as an efficient technology for mitigating escalating atmospheric CO2 levels. Porous carbons show the promising potential for CO2 capture by virtue of their tunable porosity and...
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DOI: 10.1039/D5GC03217B, PaperBinbin Chang, Weiwei Shi, Yanzhen Guo, Qixin Lu, Haitao Li, Yachao Liang, Faxue Ma, Baocheng Yang
Carbon capture has emerged as an efficient technology for mitigating escalating atmospheric CO2 levels. Porous carbons show the promising potential for CO2 capture by virtue of their tunable porosity and...
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Tracking the hydrogen spillover of heterogeneous catalysts in hydrogenation: From the formation, migration, regulation to fate
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02983J, Tutorial ReviewGuangxun Sun, Peng Xue, Lei Wang, Xin Zhang, Guangzheng Sun, Zhidong Wang, Qian Zhang, Peng Zhang, Yunqi Liu, Yuan Pan
Hydrogen spillover is a critical candidate for enhancing the hydrogenation of heterogeneous catalysts. However, the understanding and orderly controlling of spillover are still challenging. Structural design of heterogeneous catalysts significantly...
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DOI: 10.1039/D5GC02983J, Tutorial ReviewGuangxun Sun, Peng Xue, Lei Wang, Xin Zhang, Guangzheng Sun, Zhidong Wang, Qian Zhang, Peng Zhang, Yunqi Liu, Yuan Pan
Hydrogen spillover is a critical candidate for enhancing the hydrogenation of heterogeneous catalysts. However, the understanding and orderly controlling of spillover are still challenging. Structural design of heterogeneous catalysts significantly...
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Bioinspired heterogeneous catalyst for green and targeted transesterification of ethanol and dimethyl carbonate to ethyl methyl carbonate with high endurance
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC03241E, PaperRongkai Cui, Fengyue Yin, Wangquan Gong, Ningjing Yan, Siyao Li, Changshen Ye, Ting Qiu, Jie Chen
Ethyl methyl carbonate (EMC) production using transesterification of ethanol and dimethyl carbonate faces significant sustainability hurdles in conventional methods, primarily including excessive catalyst-derived solid waste and energy-intensive separations, contravening core...
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DOI: 10.1039/D5GC03241E, PaperRongkai Cui, Fengyue Yin, Wangquan Gong, Ningjing Yan, Siyao Li, Changshen Ye, Ting Qiu, Jie Chen
Ethyl methyl carbonate (EMC) production using transesterification of ethanol and dimethyl carbonate faces significant sustainability hurdles in conventional methods, primarily including excessive catalyst-derived solid waste and energy-intensive separations, contravening core...
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Sustainable base-mediated chemical upcycling of poly (propylene carbonate) to β-hydroxy sulfides and oxides
DOI: 10.1039/D5GC02451J, CommunicationNageswararao Moyilla, Ganeshdev Padhi, Nagaraju Barsu
We present a cesium carbonate–mediated method to upcycle poly(propylene carbonate) (PPC) waste into β-hydroxy sulfides, selenides, and phenoxides via selective thermal depolymerization.
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Electrochemical iron-catalyzed difunctionalization of olefins: efficient and sustainable access to β-heteroarylated esters
DOI: 10.1039/D5GC02319J, PaperBinbin Chen, Jun Xu, Zeyi Wang, Ling Yang, Qianyuan Liu, Pengfei Zhang
This study describes an electrochemical iron-catalyzed system for olefin difunctionalization with heteroarenes and methyl carbazate, providing an efficient and sustainable route to β-heteroarylated esters.
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Photo-induced C(sp3)–H functionalization of unactivated alkanes under transition-metal- and photocatalyst-free conditions
DOI: 10.1039/D5GC02386F, CommunicationYonghong Liu, Wanqiang Wang, Wei Xu, Ting Pang, Ziren Chen, Qi Xu, Xin Wang, Yonghong Zhang, Ping Liu
The Giese reaction is a powerful method for C–C bond formation, but traditional approaches typically necessitate the incorporation of a leaving group on the substrate.
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A Green Epoxidation of Unactivated Alkenes via the Catalytic Activation of Hydrogen Peroxide by 4-Hydroxybenzaldehyde
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02537K, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Efthymios T. Poursaitidis, Christiana Mantzourani, IERASIA TRIANTAFILLIDI, Maroula G Kokotou, Christoforos G Kokotos
In the quest of green, inexpensive and sustainable methods for the epoxidation of unactivated alkenes, for both academic and industrial applications, the interest in effective organocatalytic activators of hydrogen peroxide...
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DOI: 10.1039/D5GC02537K, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Efthymios T. Poursaitidis, Christiana Mantzourani, IERASIA TRIANTAFILLIDI, Maroula G Kokotou, Christoforos G KokotosIn the quest of green, inexpensive and sustainable methods for the epoxidation of unactivated alkenes, for both academic and industrial applications, the interest in effective organocatalytic activators of hydrogen peroxide...
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Predicting lignin removal efficiency in deep eutectic solvent-based biomass fractionation: an explainable machine learning approach
DOI: 10.1039/D5GC02370J, PaperZijing Zhong, Babbiker Mohammed Taher Gorish, Yue Bai, Waha Ismail Yahia Abdelmula, Wenqian Dang, Daochen Zhu
Efficient and sustainable lignin extraction is essential for advancing green biorefinery processes.
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Interfacial molecular engineering-driven self-emulsification: a green strategy for surfactant-free, high-efficiency oral delivery of cyclosporine A
DOI: 10.1039/D5GC02056E, PaperPeiya Shen, Enshi Hu, Jitong Shi, Ruipeng Li, Xingyu Zhu, Yuan Gao, Jianjun Zhang, Yuanfeng Wei, Shuai Qian
A green chemistry strategy for oral peptide delivery using biodegradable cellulose and food-grade trans-anethole enables solvent-free self-emulsification, enhancing bioavailability while minimizing environmental impact and energy use.
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The acetate anion promotes hydrolysis of poly(ethylene terephthalate) in aprotic and protic ionic liquid water mixtures
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02409A, Paper Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Maariyah Y. Suleman, Harriet Louise Judah, Panagiotis Bexis, Paul Fennell, Jason P. Hallett, Agi Brandt-Talbot
A circular plastic economy reduces raw material consumption and discourages pollution. Chemical recycling upgrades the quality of recyclate and is a complementary approach to thermomechanical recycling of plastic waste. This...
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DOI: 10.1039/D5GC02409A, Paper
Open Access   This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.Maariyah Y. Suleman, Harriet Louise Judah, Panagiotis Bexis, Paul Fennell, Jason P. Hallett, Agi Brandt-TalbotA circular plastic economy reduces raw material consumption and discourages pollution. Chemical recycling upgrades the quality of recyclate and is a complementary approach to thermomechanical recycling of plastic waste. This...
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Metal bioaccumulation prediction via QSPR-q-RASPR synergy and cross-species risk analysis
DOI: 10.1039/D5GC00904A, PaperRamin Abdullayev, Kabiruddin Khan, Gopala Krishna Jillella, Varun Gopalakrishnan Nair, Sk. Abdul Amin, Joyita Roy, Mahmoud Bousily, Agnieszka Gajewicz-Skretna
This study presents novel QSPR, q-RASPR, and SbSD models designed to predict metal bioaccumulation across a wide range of species and to identify the key molecular factors influencing this process.
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Simultaneous phenol oxygenation and quinone hydrogenation with water as both the oxygen and hydrogen source
DOI: 10.1039/D5GC01480H, PaperYongtao Wang, Kehan Yu, Wenjing Sun, Jia Yao, Haoran Li
Metal-free acid-catalyzed coupling of phenol oxygenation and 1,4-quinone hydrogenation is demonstrated using water as both the oxygen and hydrogen source, mediated by a bio-inspired geminal diol adduct.
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Engineered Pseudomonas putida monoculture system for green synthesis of 7-methylxanthine
Green Chem., 2025, Accepted Manuscript
DOI: 10.1039/D5GC02883C, PaperBhagya Sri Kolitha Jayantha, Ryan Summers, Shuyuan Zhang, Gamini P. Mendis, Lahiru N Jayakody
7-methylxanthine (7-MX) is a clinically proven safe drug to treat myopia. The chemical synthesis of 7-MX is hindered due to low specificity, demanding sustainable biological production using renewable, cost-effective feedstocks....
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DOI: 10.1039/D5GC02883C, PaperBhagya Sri Kolitha Jayantha, Ryan Summers, Shuyuan Zhang, Gamini P. Mendis, Lahiru N Jayakody
7-methylxanthine (7-MX) is a clinically proven safe drug to treat myopia. The chemical synthesis of 7-MX is hindered due to low specificity, demanding sustainable biological production using renewable, cost-effective feedstocks....
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Lignin refinement based on efficient thermo-photo-catalysis of Ru–RuO2/TiO2-deep eutectic solvents
DOI: 10.1039/D5GC02098K, PaperHekun Ding, Yue Pan, Ao Zhan, Jie Lv, Yang Yang, Zhiyuan Yang, James H. Clark, Qiang Yu
A highly effective thermo-photo-catalysis system was developed combining deep eutectic solvents (DESs) and a Ru–RuO2/TiO2 composite to enable efficient catalytic depolymerization of lignin into phenol under clean and mild conditions.
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Heterostructure of hollow MoSe2@CoSe for stable sodium storage
DOI: 10.1039/D5GC03294F, PaperKai Yang, Wenrui Zhang, Qinghua Deng, Zhiqian Li, Jiancheng Zhang, Quanli Liu, Hao Mo, Nan Zhu
An exquisite hierarchical heterostructure of MoSe2@CoSe significantly promotes sodium-ion storage kinetics, lowers the ion diffusion barrier, and improves structural stability during long-life cycles.
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Kinetic-control difunctionalization of olefins to α-hydroxycarbonyls under catalyst-free conditions
DOI: 10.1039/D5GC02308D, Communication
Open Access 
  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Hong-Yu Hou, Yuan-Yuan Cheng, Xin-Yu Zhang, Ke Zhang, Hui-Zhen Ren, Kaiyi Su, Zhiyuan Huang, Bin Chen, Chen-Ho Tung, Li-Zhu WuCatalyst-free difunctionalization of alkene is achieved under visible light irradiation to form complex α-hydroxycarbonyls.
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Electroenzymatic cascade synthesis of 2,3-diaminophenazine on HRP-ZnGa2O4 nano-biohybrids
DOI: 10.1039/D5GC03726C, PaperYuxuan Cheng, Zhe Wang, Siqi Li, Meixuan Li, Shuni Li, Xue Xiao, Yucheng Jiang, Yu Chen
In this work, a novel nano-biohybrid has been developed for the efficient synthesis of 2,3-diaminophenazine (DAP), a biologically significant heterocyclic compound, via an electroenzymatic cascade catalysis system.
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Advancing lignocellulosic conversion though biosensor-enabled metabolic engineering
DOI: 10.1039/D5GC03618F, Tutorial Review
Open Access   This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.Qi Gan, Jianli Zhang, Xinyu Gong, Yusong Zou, Yajun YanBiosensor-aided metabolic engineering is advancing the conversion of lignocellulosic biomass by enabling regulation and optimization of microbial production pathways.
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